| Download | - View final version: First-order melting of a weak spin-orbit Mott insulator into a correlated metal (PDF, 990 KB)
|
|---|
| DOI | Resolve DOI: https://doi.org/10.1103/PhysRevLett.114.257203 |
|---|
| Author | Search for: Hogan, Tom; Search for: Yamani, Z.1; Search for: Walkup, D.; Search for: Chen, Xiang; Search for: Dally, Rebecca; Search for: Ward, Thomas Z.; Search for: Dean, M. P. M.; Search for: Hill, John; Search for: Islam, Z.; Search for: Madhavan, Vidya; Search for: Wilson, Stephen D. |
|---|
| Name affiliation | - National Research Council of Canada. Security and Disruptive Technologies
|
|---|
| Format | Text, Article |
|---|
| Subject | Magnetic susceptibility; Phase separation Antiferromagnetics; Electronic phase diagram; First-order melting; La substitutions; Mott insulators; Nano-scale phase separation; Spin susceptibility; Structural distortions |
|---|
| Abstract | The electronic phase diagram of the weak spin-orbit Mott insulator (Sr₁−xLax)₃Ir₂O₇ is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a narrow regime of nanoscale phase separation comprised of antiferromagnetic, insulating regions and paramagnetic, metallic puddles persisting until x≈0.04. Continued electron doping results in an abrupt, first-order phase boundary where the Néel state is suppressed and a homogenous, correlated, metallic state appears with an enhanced spin susceptibility and local moments. As the metallic state is stabilized, a weak structural distortion develops and suggests a competing instability with the parent spin-orbit Mott state. |
|---|
| Publication date | 2015-06-25 |
|---|
| Publisher | American Physical Society |
|---|
| In | |
|---|
| Language | English |
|---|
| Peer reviewed | Yes |
|---|
| NPARC number | 23001058 |
|---|
| Export citation | Export as RIS |
|---|
| Report a correction | Report a correction (opens in a new tab) |
|---|
| Record identifier | 52705cc0-e17a-4735-a2b2-c0250cf7e564 |
|---|
| Record created | 2016-12-06 |
|---|
| Record modified | 2020-06-02 |
|---|
