| Download | - View accepted manuscript: Femtosecond Coulomb explosion imaging of vibrational wave functions (PDF, 551 KiB)
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| DOI | Resolve DOI: https://doi.org/10.1103/PhysRevLett.82.3416 |
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| Author | Search for: Chelkowski, S.; Search for: Corkum, P. B.1; Search for: Bandrauk, A. D. |
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| Affiliation | - National Research Council of Canada. Security and Disruptive Technologies
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| Format | Text, Article |
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| Abstract | Because of the nonlinearity of multiphoton ionization, an intense 5 fs pulse is short enough to change the ionization probability from near zero to near unity in less than one-half of a laser period. For H₂⁺ this exposes all parts of the vibrational wave function to the full force of Coulomb repulsion at nearly the same time. By solving the time dependent Schrödinger equation, following both electron and ion motion we show that the initial vibrational wave function Ψ(R) of H₂⁺ can be reconstructed by using Coulomb's law to map the ion fragment kinetic energy spectrum into |Ψ(R)|². |
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| Publication date | 1999-04-26 |
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| In | |
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| Language | English |
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| Peer reviewed | Yes |
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| NPARC number | 21277558 |
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| Export citation | Export as RIS |
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| Report a correction | Report a correction (opens in a new tab) |
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| Record identifier | e9bcd590-48a0-4e6b-90b9-611d6e475b87 |
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| Record created | 2016-04-18 |
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| Record modified | 2020-06-04 |
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