Observing molecular dynamics with timed Coulomb explosion imaging

From National Research Council Canada

DOIResolve DOI: https://doi.org/10.1098/rsta.1998.0168
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Name affiliation
  1. National Research Council Canada
  2. National Research Council Canada. NRC Steacie Institute for Molecular Sciences
  3. National Research Council Canada. Security and Disruptive Technologies
FormatText
TypeArticle
Journal titlePhilosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences
ISSN1364-503X
1471-2962
Volume356
Issue1736
Pages329–344; # of pages: 16
SubjectCoulomb explosion imaging; molecular structure; femtosecond pump-probe technique; imaging methods; pump-probe technique
Abstract
The Coulomb explosion method for imaging molecular structure is combined with the femtosecond pump–probe technique. Thus the imaging method becomes flexible enough to determine molecular structure even in highly excited or transient states as a function of time. Examples for the applicability of this method are given. The major concerns which could limit the reliability and the accuracy of the information extracted are discussed and solutions proposed. In addition to observing time–dependent structures, optically triggered Coulomb explosion imaging can be used to identify unusual events in an ensemble of common but more frequent events.
Publication date
PublisherThe Royal Society Publishing
LanguageEnglish
NPARC number21277565
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