| DOI | Resolve DOI: https://doi.org/10.1103/PhysRevLett.98.187402 |
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| Author | Search for: Dietzek, Benjamin; Search for: Gräfe, Stefanie1; Search for: Schmitt, Michael; Search for: Yartsev, Arkady; Search for: Pascher, Torbjörn; Search for: Sundström, Villy; Search for: Kiefer, Wolfgang; Search for: Ivanov, Misha Yu1 |
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| Affiliation | - National Research Council of Canada. NRC Steacie Institute for Molecular Sciences
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| Format | Text, Article |
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| Subject | dielectric materials; optical phase matching; stimulated Raman scattering; vibrational modes |
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| Abstract | We use high-order Raman scattering in a bulk dielectric to characterize coherent dynamics with precision typical for gas phase experiments. The experimental pump-probe approach allows for the simultaneous observation and separation in space and time of the individual contributions of different-order Raman processes to a coherent wave packet without relying on phase-matching conditions and within the same experimental geometry. We propose a novel technique to discriminate between stimulated excitation of vibronic levels in the impulsive and intermediate excitation regimes, futhermore allowing us to distinguish between different pathways contributing to the same fifth-order Raman processes. |
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| Publication date | 2007-05-04 |
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| In | |
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| Language | English |
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| NPARC number | 12339117 |
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| Export citation | Export as RIS |
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| Report a correction | Report a correction (opens in a new tab) |
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| Record identifier | 3e55f85b-9468-484b-ac6b-c6208ba9c017 |
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| Record created | 2009-09-11 |
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| Record modified | 2020-05-10 |
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