| Abstract | Flexible strain sensors have seen significant development for applications in human–machine interfaces (HMI), soft robotics, and wearable electronics. However, issues like conformability, reusability, customizability, and long-term stretchability remain. This paper introduces a customizable, self-adaptive, and biocompatible wearable strain sensor made from polyvinyl alcohol (PVA), silk fibroin (SF), and multi-walled carbon nanotubes (MWCNT) for wearable motion sensing. Inspired by the viscoelastic behaviour of Silly Puttyᵀᴹ, we incorporated hygroscopic calcium chloride (CaCl₂) to allow the sensor to absorb ambient moisture and adapt to any arbitrary surface geometries while maintaining its stretchability and sensitivity without needing adhesives. Using direct ink writing (DIW), desirable sensor geometries can be created for targeted on-body strain monitoring. A computational method is applied to identify the printing pressure and temperature ranges for optimal printability. Further, the developed sensors can be applied in a tattoo-like fashion that can be directly transfer-printed onto a suitable surface. Cyclic loading, high strain loading, and finite element analysis validated ideal conformability between the tattoo sensor and the body surface. Additionally, it is demonstrated that the developed sensor can be printed in a modular configuration, such as multiple single-line patterns. These patterns can then be assembled and personalized based on the user’s anatomy, the direction of movement, and specific functional requirements. This flexibility allows the sensor to be tailored to each application, considering all limitations and necessities, making it highly customizable. The PVA-SF-MWCNT sensor further offers exceptional longevity, self-healability, and reusability to accommodate unique wearable HMI application needs. |
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